This idea came from watching the original Saturday morning cartoon run of episodes and Friday Night Videos, the NBC late night show that featured 90 minutes of videos on regular TV before people got their MTV...the idea of creating an SMTV (Smurf Music Television) of sorts where popular music and Smurf cartoons would blend together, creating an interesting mix. Here's a collection of suggestions that came from the top of my head:
| Band or Musician | Song Name | Cartoon Episode | Comments |
| Ace Of Base | "The Sign" | "Smurfing In Sign Language" | |
| Aerosmith | "Dude Looks Like A Lady" | "Smurfette For A Day" | |
| The Beatles | "Help" | Any episode where a Smurf has to be rescued | |
| The Beatles | "Octopus' Garden" | "Handy's Sweetheart" and any underwater-based episodes | |
| Pat Benatar | "Hit Me With Your Best Shot" | "The Masked Pie Smurfer" | |
| Bow Wow Wow | "Candy" | "Smurfette's Sweet Tooth" | |
| Lindsey Buckingham | "Holiday Road" | "Smurfs On Wheels" | From the National Lampoon's Vacation series of movies |
| Peter Cetera | "For The Glory Of Love" | "Don Smurfo" | From the motion picture The Karate Kid Part 2 |
| Phil Collins | "Against All Odds" | "Handy's Sweetheart" | It's appropriate for a mismatched love relationship! |
| Phil Collins | "Take Me Home" | Episodes where a Smurf is stuck on some island in need of rescue | |
| The Cowsills | "Hair" | "Smurfette's Golden Tresses", "Symbols Of Wisdom" | From the musical Hair |
| Culture Club | "The War Song" | "All's Smurfy That Ends Smurfy" | |
| Def Leppard | "Animal" | "Brainy's Beastly Boo-Boo" | |
| Sheena Easton | "Telefone" | "The First Telesmurf" | |
| Electric Light Orchestra | "Turn To Stone" | "Petrified Smurfs" | |
| Gloria Estefan | "Coming Out Of The Dark" | "The Dark-Ness Monster" | |
| Gloria Estefan | "Reach" | "The Smurfic Games" | |
| Eurhthymics with Aretha Franklin | "Sisters Are Doing It For Themselves" | "Sister Smurf", "Sassette" | |
| The Fabulous Thunderbirds | "Tough Enough" | Episodes where Hefty or Tuffy go out of their way to prove themselves | |
| The Fifth Dimension | "(Last Night) I Didn't Get To Sleep" | "Things That Go Smurf In The Night", "Sleepless Smurfs" | |
| The Fifth Dimension | "Up, Up, And Away" | "Handy's Kite" | |
| A Flock Of Seagulls | "Burnin' Up" | "Clockwork's Power Play" | |
| A Flock Of Seagulls | "I Ran (So Far Away)" | "The Fastest Wizard In The World" | |
| A Flock Of Seagulls | "You Can Run" | Chase sequences | |
| Filter | "Take A Picture" | "Shutterbug Smurfs" | |
| Five For Fighting | "Superman (It's Not Easy)" | "Supersmurf", "Breakfast At Greedy's" | The latter episode because of the Smurfs uncontrollably floating around |
| The Fixx | "One Thing Leads To Another" | "Predictable Smurfs" | |
| The Fixx | "Red Skies At Night" | "Lost Smurf" | Fits in with the color-cycling skies that appeared with the emergence of Castle Captive |
| The Fixx | "Saved By Zero" | "Nobody Smurf" | |
| Frankie Goes To Hollywood | "Two Tribes" | "Big Shot Smurfs", "The Smurfic Games" | |
| Peter Gabriel | "Big Time" | "Little Big Smurf" | |
| Genesis | "Invisible Touch" | "Jokey's Cloak" | |
| The Go-Gos | "Head Over Heels" | "Reckless Smurfs" | |
| The Grateful Dead | "A Touch Of Grey" | "The Color Smurfy" | |
| The Guess Who | "No Time Left" | "No Time For Smurfs" | |
| Sammy Hagar | "I Can't Drive 55" | "The Smurfbox Derby" | |
| Daryl Hall & John Oates | "I Can't Go For That (No Can Do)" | "The Smurf Who Couldn't Say No" | |
| Hanson | "Mmmbop" | "The Smurflings" | The Hansons in that song sound like Smurflings |
| Don Henley | "Dirty Laundry" | "All The News That's Fit To Smurf" | |
| Whitney Houston | "One Moment In Time" | "The Smurfic Games" | |
| Billy Idol | "Dancing With Myself" | "Jungle Jitterbugs" | |
| Billy Idol | "Eyes Without A Face" | "Grandpa's Nemesis" | |
| INXS | "Devil Inside" | Any episode where a Smurf has the Devil Smurf and Angel Smurf appear alongside them to help them make a decision | |
| INXS | "Disappear" | "The Kaplowey Scroll" | |
| INXS | "Kick" | "Smurf The Other Cheek" | |
| Michael Jackson | "Man In The Mirror" | Episodes involving Vanity and his mirror | |
| Michael Jackson & Paul McCartney | "The Girl Is Mine" | "Romeo And Smurfette" | Fits with the feuding between Handy and Hefty |
| The J. Geils Band | "Freeze Frame" | "Shutterbug Smurfs" | |
| Billy Joel | "An Innocent Man" | "The Smurfy Verdict" | |
| Billy Joel | "Pressure" | "Tick-Tock Smurfs" | |
| Billy Joel | "Tell Her About It" | "Speak For Yourself Farmer Smurf" | |
| Billy Joel | "We Didn't Start The Fire" | "Fire Fighting Smurfs" | |
| Elton John | "Rocket Man" | "The Astrosmurf" | |
| Kansas | "Play The Game Tonight" | "The Grouchiest Game In Town" | |
| Kansas | "Point Of Know Return" | "The Smurf Who Would Be King" | |
| Kiss | "I" | "A Little Smurf Confidence" | From the album Music From The Elder |
| Kiss | "Tears Are Falling" | "The Tear Of A Smurf" | |
| Patti LaBelle | "Burning Up" | "Clockwork's Power Play" | |
| Cyndi Lauper | "Change Of Heart" | "Hefty's Heart" | |
| Cyndi Lauper | "True Colors" | "The Color Smurfy" | |
| Huey Lewis & The News | "Back In Time" | The 1989-1990 season of episodes | From the motion picture Back To The Future |
| Madonna | "Frozen" | "S-Shivering S-Smurfs" | |
| Madonna | "Little Star" | "Once In A Blue Moon" | |
| Madonna | "Lucky Star" | "Smurfette's Lucky Star" | |
| Madonna | "Music" | Any music-related episode | |
| Madonna | "The Power Of Goodbye" | "Squeaky" | |
| Madonna | "Ray Of Light" | "Clumsy's Cloud" | |
| Madonna | "Who's That Girl" | "The Smurfette", "Smurfette Unmade" | |
| Men At Work | "Down Under" | "G'Day Smoogle" | |
| Men Without Hats | "Antarctica" | "No Reflection On Vanity" | |
| Men Without Hats | "I Like" | Any episode where Brainy tries to apply his intelligence to a situation, which fails him and others | |
| Men Without Hats | "Living In China" | "Imperial Panda-Monium" | |
| Men Without Hats | "The Safety Dance" | "The Hundredth Smurf" | Papa Smurf has his little Smurfs perform this "Dance of 100 Smurfs" to counter a spell of bad luck |
| Freddie Mercury | "Living On My Own" | "Dreamy's Nightmare" | |
| Freddie Mercury | "Mr. Bad Guy" | No particular episode, but a good character song for the likes of Gargamel | |
| Bette Midler | "The Rose" | "Smurfette's Rose" | From the motion picture of the same name |
| Milli Vanilli | "Blame It On The Rain" | "Blue Eyes Returns" | |
| The Miracles | "Love Machine" | "Clockwork Smurfette" | |
| The Monkees | "I'm A Believer" | "The Smurfette", "Romeo And Smurfette" | |
| Nena | "99 Red Balloons" | "The Purple Smurfs" | Maybe a parody version; "99 purple Smurfs hopping up and down my turf,..." |
| Billy Ocean | "The Color Of Love" | "Every Picture Smurfs A Story" | |
| Oingo Boingo | "Weird Science" | "The Smurfette", "Clockwork Smurfette" | From the motion picture Weird Science |
| Tom Petty | "I Won't Back Down" | "The Smurf Who Couldn't Say No" | |
| Tom Petty & The Heartbreakers | "It's Good To Be King" | "King Smurf" | |
| The Police | "Walking On The Moon" | "The Man In The Moon" | |
| Queen | "I Want It All" | "The Smurfs And The Money Tree" | |
| R.E.M. | "Everybody Hurts" | "Crying Smurfs" | |
| R.E.M. | "It's The End Of The World As We Know It" | "The Comet Is Coming" | |
| R.E.M. | "Man On The Moon" | "The Man In The Moon" | |
| Rockwell | "Somebody's Watching Me" | "Haunted Smurfs", "Smurfing For Ghosts" | |
| Savage Garden | "I Knew I Loved You" | "Smurfily Ever After" | This would also be a great song for the wedding of Empath and Smurfette |
| Savage Garden | "The Animal Song" | "Smurf On The Wild Side" | |
| Peter Schilling | "Major Tom" | "The Astrosmurf" | |
| Simon & Garfunkel | "The Sound Of Silence" | "Unsound Smurfs" | |
| Soul Asylum | "Runaway Train" | "Locomotive Smurfs" | |
| Bruce Springsteen | "Brilliant Disguise" | "The Fake Smurf", "The Baby Smurf", and pretty much any episode involving masquerading villains | |
| Bruce Springsteen | "Going Down" | "The Incredible Shrinking Wizard" | |
| Amii Stewart | "Knock On Wood" | "Smurf On Wood" | |
| Rod Stewart | "Forever Young" | "Grandpa's Fountain Of Youth" | |
| Styx | "Mr. Roboto" | "The Clockwork Smurf" | |
| Styx | "Come Sail Away" | Episodes featuring Dreamy as captain of the S.S. Smurf | |
| Thompson Twins | "Doctor, Doctor" | "Calling Dr. Smurf" | |
| Thompson Twins | "Hold Me Now" | "A Hug For Grouchy" | |
| Thompson Twins | "King For A Day" | "King Smurf", "Queen Smurfette" | |
| Thompson Twins | "Lies" | "The Whole Smurf And Nothing But The Smurf", "Smurfs On The Run" | |
| Twisted Sister | "We're Not Gonna Take It" | "The Masked Pie Smurfer", "Greedy Goes On Strike" | |
| The Waitresses | "I Know What Boys Like" | "Romeo And Smurfette" | |
| Anita Ward | "Ring My Bell" | "A Bell For Azrael" | |
| Dionne Warwick | "That's What Friends Are For" | "The Smurfiest Of Friends" | |
| Vanessa Williams | "Colors Of The Wind" | "How To Smurf A Rainbow" | From the Disney motion picture Pocahontas |
| Weird Al Yankovic | "Eat It" | "Greedy And The Porridge Pot" | |
| Weird Al Yankovic | "Fat" | "Gormandizing Greedy" and any episode that Bigmouth appears in | |
| Weird Al Yankovic | "I Love Rocky Road" | "The Smurfwalk Cafe" | A parody of Joan Jett & The Blackheart's "I Love Rock & Roll" |
| Weird Al Yankovic | "Like A Surgeon" | "Jokey's Funny Bone" | |
| Weird Al Yankovic | "Slime Creatures From Outer Space" | "The Bad Place" | |
| Weird Al Yankovic | "You Think I'm A Clone Now" | "Smurfiplication", "A Maze Of Mirrors" | A parody of Tiffany's "I Think We're Alone Now" |